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  1. Heterostructures of ferromagnetic (FM) and noble metal (NM) thin films have recently attracted considerable interest as viable platforms for the ultrafast generation, control, and transduction of light-induced spin currents. In such systems, an ultrafast laser can generate a transient spin current in the FM layer, which is then converted to a charge current at the FM/NM interface due to strong spin–orbit coupling in the NM layer. Whether such conversion can happen in a single material and how the resulting spin current can be quantified are open questions under active study. Here, we report ultrafast THz emission from spin–charge conversion in a bare FeRh thin film without any NM layer. Our results highlight that the magnetic material by itself can enable spin–charge conversion in the same order as that in a FM/NM heterostructure. We further propose a simple model to estimate the light-induced spin current in FeRh across its metamagnetic phase transition temperature. Our findings have implications for the study of the ultrafast dynamics of magnetic order in quantum materials using THz emission spectroscopy.

     
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    Free, publicly-accessible full text available April 18, 2025
  2. Binary kagome compounds TmXn (T = Mn, Fe, Co; X = Sn, Ge; m:n = 3:1, 3:2, 1:1) have garnered recent interest owing to the presence of both topological band crossings and flatbands arising from the geometry of the metal-site kagome lattice. To exploit these electronic features for potential applications in spintronics, the growth of high-quality heterostructures is required. Here, we report the synthesis of Fe/FeSn and Co/FeSn bilayers on Al2O3 substrates using molecular beam epitaxy to realize heterointerfaces between elemental ferromagnetic metals and antiferromagnetic kagome metals. Structural characterization using high-resolution x-ray diffraction, reflection high-energy electron diffraction, and electron microscopy reveals that the FeSn films are flat and epitaxial. Rutherford backscattering spectroscopy was used to confirm the stoichiometric window where the FeSn phase is stabilized, while transport and magnetometry measurements were conducted to verify metallicity and magnetic ordering in the films. Exchange bias was observed, confirming the presence of antiferromagnetic order in the FeSn layers, paving the way for future studies of magnetism in kagome heterostructures and potential integration of these materials into devices.

     
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    Free, publicly-accessible full text available February 28, 2025
  3. Free, publicly-accessible full text available March 15, 2025
  4. Abstract

    The confluence between high-energy physics and condensed matter has produced groundbreaking results via unexpected connections between the two traditionally disparate areas. In this work, we elucidate additional connectivity between high-energy and condensed matter physics by examining the interplay between spin-orbit interactions and local symmetry-breaking magnetic order in the magnetotransport of thin-film magnetic semimetal FeRh. We show that the change in sign of the normalized longitudinal magnetoresistance observed as a function of increasing in-plane magnetic field results from changes in the Fermi surface morphology. We demonstrate that the geometric distortions in the Fermi surface morphology are more clearly understood via the presence of pseudogravitational fields in the low-energy theory. The pseudogravitational connection provides additional insights into the origins of a ubiquitous phenomenon observed in many common magnetic materials and points to an alternative methodology for understanding phenomena in locally-ordered materials with strong spin-orbit interactions.

     
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  5. Nonreciprocal magnon propagation has recently become a highly potential approach of developing chip-embedded microwave isolators for advanced information processing. However, it is challenging to achieve large nonreciprocity in miniaturized magnetic thin-film devices because of the difficulty of distinguishing propagating surface spin waves along the opposite directions when the film thickness is small. In this work, we experimentally realize unidirectional microwave transduction with sub-micrometer-wavelength propagating magnons in a yttrium iron garnet (YIG) thin-film delay line. We achieve a non-decaying isolation of 30 dB with a broad field-tunable bandpass frequency range up to 14 GHz. The large isolation is due to the selection of chiral magnetostatic surface spin waves with the Oersted field generated from the coplanar waveguide antenna. Increasing the geometry ratio between the antenna width and YIG thickness drastically reduces the nonreciprocity and introduces additional magnon transmission bands. Our results pave the way for on-chip microwave isolation and tunable delay line with short-wavelength magnonic excitations.

     
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    Free, publicly-accessible full text available July 10, 2024
  6. Free, publicly-accessible full text available October 1, 2024
  7. Synthetic antiferromagnet (SAF) nanostructures with an interfacial Dzyaloshinskii–Moriya interaction can host topologically distinct spin textures, such as skyrmions, and therefore, are regarded as promising candidates for both spintronics and magnonics applications. Here, we present comprehensive micromagnetic simulations of such material systems and discuss the rich phase diagrams that contain various types of magnetic configurations. Aside from the static properties, we further discuss the resonant excitations of the calculated magnetic states, which include individual skyrmions and skyrmioniums. Finally, the internal modes of SAF skyrmion clusters are studied and discussed in the context of magnetic sensing applications based on the dynamic fingerprint in broadband ferromagnetic resonance measurements. 
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  8. Materials with large spin–orbit interactions generate pure spin currents with spin polarizations parallel to the interfacial surfaces that give rise to conventional spin–orbit torques. These spin–orbit torques can only efficiently and deterministically switch magnets with in-plane magnetization. Additional symmetry breaking, such as in non-collinear antiferromagnets, can generate exotic, unconventional spin–orbit torques that are associated with spin polarizations perpendicular to the interfacial planes. Here, we use micromagnetic simulations to investigate whether such exotic spin–orbit torques can generate magnetic droplet solitions in out-of-plane magnetized geometries. We show that a short, high current pulse followed by a lower constant current can nucleate and stabilize magnetic droplets. Through specific current pulse lengths, it is possible to control the number of droplets in such a system, since torques are generated over a large area. Additionally, the nucleation current scales with the out-of-plane component of the spin polarization and is linear as a function of magnetic field strength. 
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